Manganese-Catalyzed Hydrocarbofunctionalization of Internal Alkenes
Chinese Journal of Chemistry, ISSN: 1614-7065, Vol: 38, Issue: 12, Page: 1497-1502
2020
- 23Citations
- 6Captures
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Example: if you select the 1-year option for an article published in 2019 and a metric category shows 90%, that means that the article or review is performing better than 90% of the other articles/reviews published in that journal in 2019. If you select the 3-year option for the same article published in 2019 and the metric category shows 90%, that means that the article or review is performing better than 90% of the other articles/reviews published in that journal in 2019, 2018 and 2017.
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Article Description
A highly regio- and chemo-selective dimeric Mn(I)-catalyzed hydroarylation and hydroalkenylation of unbiased internal alkenes with commercially abundant organoboron compounds is reported. A wide range of densely functionalized aliphatic alkenyl amides can successfully undergo site-exclusive hydrocarbofunctionalization in air atmosphere without any exogenous directing auxiliary, affording an enhanced lead library of structurally diverse γ-functionalized carboxylic acid derivatives in moderate to good yields. The precise chemoselectivity of the reaction among multiple alkene units even in the presence of reactive terminal alkenes highlights the unique catalytic features of manganese catalyst, and the excellent functional group compatibility of primary amides further complements other transition metals.
Bibliographic Details
http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=85090311021&origin=inward; http://dx.doi.org/10.1002/cjoc.202000376; https://onlinelibrary.wiley.com/doi/10.1002/cjoc.202000376; https://dx.doi.org/10.1002/cjoc.202000376; http://sciencechina.cn/gw.jsp?action=cited_outline.jsp&type=1&id=6866848&internal_id=6866848&from=elsevier
Wiley
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