Interfacial charge-transfer loss in dye-sensitized solar cells
Journal of Physical Chemistry C, ISSN: 1932-7447, Vol: 117, Issue: 6, Page: 2734-2739
2013
- 15Citations
- 32Captures
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Article Description
Interfacial charge-transfer loss factors (CTLFs) of dye-sensitized solar cells (DSCs) were studied using a thermionic emission-diffusion theory and electrochemical impedance spectroscopy (EIS). It is found that the subsidiary CTLFs can be quantified including a native charge-transfer loss at the TiO /electrolyte interface in DSC devices. The obtained CTLFs as a probability parameter α were identified as almost matching to dominant resistance-capacitance (RC) time constants obtained from the EIS and its numerical calculation. The quantified CTLFs based on a detailed physical model of quantum-mechanical tunneling and reflection of charge carriers can explain a degradation of open-circuit voltage in DSC devices. © 2013 American Chemical Society.
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