Ni or Ru supported on MgO/γ-AlO pellets for the catalytic conversion of ethanol into butanol
RSC Advances, ISSN: 2046-2069, Vol: 8, Issue: 45, Page: 25846-25855
2018
- 24Citations
- 34Captures
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Example: if you select the 1-year option for an article published in 2019 and a metric category shows 90%, that means that the article or review is performing better than 90% of the other articles/reviews published in that journal in 2019. If you select the 3-year option for the same article published in 2019 and the metric category shows 90%, that means that the article or review is performing better than 90% of the other articles/reviews published in that journal in 2019, 2018 and 2017.
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Metrics Details
- Citations24
- Citation Indexes24
- 24
- CrossRef19
- Captures34
- Readers34
- 34
Article Description
Ni- and Ru-based catalytic pellets supported on commercial γ-AlO pellets modified with magnesium oxide have been prepared for application in the catalytic conversion of ethanol into butanol. MgO/γ-AlO pellets with or without added metals have been characterized by XRD, SEM/EDX, TGA, N physisorption, H TPR, and CO TPD in order to investigate the effect of MgO coverage and metal distribution on the surface and red-ox properties of the materials and, in turn, their effects on the catalytic performance. The conversion of ethanol into butanol has been investigated in a continuous flow reactor at 350-400 °C under diluted conditions (3% ethanol) in order to rank the different catalytic pellets and identify the best formulations and preparation procedures via a comparison with powder catalysts previously proposed in the literature with similar compositions. Results show enhanced catalytic performance for MgO-covered alumina pellets with respect to a pure MgO powder catalyst in spite of the lower MgO load. A significant further positive effect is found when Ni or Ru enters a solid solution with MgO.
Bibliographic Details
http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=85050377264&origin=inward; http://dx.doi.org/10.1039/c8ra04310h; http://www.ncbi.nlm.nih.gov/pubmed/35539807; https://xlink.rsc.org/?DOI=C8RA04310H; https://dx.doi.org/10.1039/c8ra04310h; https://pubs.rsc.org/en/content/articlelanding/2018/ra/c8ra04310h
Royal Society of Chemistry (RSC)
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