Hierarchical Chitin Fibers with Aligned Nanofibrillar Architectures: A Nonwoven-Mat Separator for Lithium Metal Batteries.

Citation data:

ACS nano, ISSN: 1936-086X, Vol: 11, Issue: 6, Page: 6114-6121

Publication Year:
2017
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Repository URL:
http://scholarworks.unist.ac.kr/handle/201301/21974
PMID:
28505417
DOI:
10.1021/acsnano.7b02085
Author(s):
Kim, Joong-Kwon; Kim, Do Hyeong; Joo, Se Hun; Choi, Byeongwook; Cha, Aming; Kim, Kwang Min; Kwon, Tae-Hyuk; Kwak, Sang Kyu; Kang, Seok Ju; Jin, Jungho
Publisher(s):
American Chemical Society (ACS); AMER CHEMICAL SOC
Tags:
Materials Science; Engineering; Physics and Astronomy; chitin fiber; DEMS; Li dendrite; Li− O2 battery; separator
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article description
Here, we introduce regenerated fibers of chitin (Chiber), the second most abundant biopolymer after cellulose, and propose its utility as a nonwoven fiber separator for lithium metal batteries (LMBs) that exhibits an excellent electrolyte-uptaking capability and Li-dendrite-mitigating performance. Chiber is produced by a centrifugal jet-spinning technique, which allows a simple and fast production of Chibers consisting of hierarchically aligned self-assembled chitin nanofibers. Following the scrutinization on the Chiber-Li-ion interaction via computational methods, we demonstrate the potential of Chiber as a nonwoven mat-type separator by monitoring it in Li-O and Na-O cells.