Nucleation and Growth Mechanism of Anion-Derived Solid Electrolyte Interphase in Rechargeable Batteries
Angewandte Chemie - International Edition, ISSN: 1521-3773, Vol: 60, Issue: 15, Page: 8521-8525
2021
- 94Citations
- 54Captures
- 5Mentions
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Metrics Details
- Citations94
- Citation Indexes94
- 94
- CrossRef60
- Captures54
- Readers54
- 54
- Mentions5
- News Mentions4
- News4
- Blog Mentions1
- Blog1
Most Recent News
Anions and solvents direct nucleation and growth of the solid electrolyte interphase
Batteries charge and recharge—apparently all thanks to a perfect interplay of electrode material and electrolyte. However, for ideal battery function, the solid electrolyte interphase (SEI) plays a crucial role. Materials scientists have now studied nucleation and growth of this layer in atomic detail. According to the study published in the journal Angewandte Chemie, the properties of anions and
Article Description
Solid electrolyte interphase (SEI) has been widely employed to describe the new phase formed between anode and electrolyte in working batteries. Significant advances have been achieved on the structure and composition of SEI as well as on the possible ion transport mechanism. However, the nucleation and growth mechanism of SEI catches little attention, which requires the establishment of isothermal electrochemical crystallization theory. Herein we explore the virgin territory of electrochemically crystallized SEI. By using potentiostatic method to regulate the decomposition of anions, an anion-derived SEI forms on graphite surface at atomic scale. After fitting the cur-rent-time transients with Laviron theory and Avrami formula, we conclude that the formation of anion-derived interface is surface reaction controlled and obeys the two-dimensional (2D) progressive nucleation and growth model. Atomic force microscope (AFM) images emphasize the conclusion, which reveals the mystery of isothermal electrochemical crystallization of SEI.
Bibliographic Details
Wiley
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