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Cu NMR in the normal state of HgBaCaCuO

Journal of Low Temperature Physics, ISSN: 0022-2291, Vol: 105, Issue: 3-4, Page: 371-376
1996
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We present a Cu NMR study of HgBaCaCuO underdoped single crystals with T ≃ 115 K. While the uniform spin susceptibility decreases below T ≃ 370 K, relaxation rate measurements demonstrate the opening of a spin-gap at Q = (π, π) below T* ≃ 230 K, the highest temperature reported so far. The characteristic energy of spin fluctuations is shown to be higher than in underdoped YBaCuO and the analysis of the quadrupole and hyperfine couplings suggests that the in-plane Cu-O hybridization is also stronger. The T-dependence of T is the same in the three CuO planes which seems hardly compatible with the pure interlayer spin-pairing picture. © 1996 Plenum Publishing Corporation.

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