Linear and non-linear response of embedded Na clusters
Applied Physics A: Materials Science and Processing, ISSN: 0947-8396, Vol: 82, Issue: 1 SPEC. ISS., Page: 151-159
2006
- 20Citations
- 10Captures
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Article Description
We investigate Na clusters embedded in Ar matrices. The surrounding Ar atoms are modeled in terms of their dynamical polarizability and the strong electron repulsion. The calibration of the model is discussed. First results for the non-linear optical response of the Na clusters are presented for the test case of Na embedded in Ar ensembles of different sizes. It is shown that blue shift through core repulsion and red shift through dipole polarizability counterweight each other to the end that very little global shift is seen in the spectra. This feature persists to all excitation strengths considered. There are, however, detailed effects, such as for example the Landau fragmentation of the Mie plasmon peak.
Bibliographic Details
http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=29144498253&origin=inward; http://dx.doi.org/10.1007/s00339-005-3353-7; http://link.springer.com/10.1007/s00339-005-3353-7; http://link.springer.com/content/pdf/10.1007/s00339-005-3353-7; http://link.springer.com/content/pdf/10.1007/s00339-005-3353-7.pdf; http://link.springer.com/article/10.1007/s00339-005-3353-7/fulltext.html; https://dx.doi.org/10.1007/s00339-005-3353-7; https://link.springer.com/article/10.1007/s00339-005-3353-7; http://www.springerlink.com/index/10.1007/s00339-005-3353-7; http://www.springerlink.com/index/pdf/10.1007/s00339-005-3353-7
Springer Science and Business Media LLC
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