Multifunctional NiCoTi Catalyst Derived from Layered Double Hydroxides for Selective Hydrogenation of 5-Hydroxymethylfurfural to 2,5-Dimethylfuran
Catalysis Letters, ISSN: 1572-879X, Vol: 151, Issue: 2, Page: 517-525
2021
- 16Citations
- 16Captures
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Article Description
Multifunctional NiCoTi metal oxide catalysts (denoted herein as NiCoTi-x, where x is the molar ratio Ni + Co:Ti) were successfully prepared by thermal treatment of NiCoTi layered double hydroxide (LDH) precursors. The NiCoTi-x catalysts were then applied to the hydrogenation of 5-hydroxymethylfurfural (HMF) to 2,5-dimethylfuran (DMF). The Ni:Co:Ti molar ratio in the catalysts was found to strongly influence both catalyst activity and product selectivity. A NiCoTi-8 catalyst, containing Ni, Co and Ti in a 4:4:1 molar ratio (i.e. Ni + Co/Ti = 8), displayed outstanding performance for HMF hydrogenation at 200 °C and 1.5 MPa, evidenced by a 90.7% HMF conversion and 95.8% selectivity to DMF. Graphic Abstract: A ternary metal oxide catalyst derived from a layered double hydroxide was proposed for the efficient and selective hydrogenation of 5-hydroxymethylfurfural to 2,5-methylfuran.[Figure not available: see fulltext.]
Bibliographic Details
http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=85088431952&origin=inward; http://dx.doi.org/10.1007/s10562-020-03323-8; https://link.springer.com/10.1007/s10562-020-03323-8; https://link.springer.com/content/pdf/10.1007/s10562-020-03323-8.pdf; https://link.springer.com/article/10.1007/s10562-020-03323-8/fulltext.html; https://dx.doi.org/10.1007/s10562-020-03323-8; https://link.springer.com/article/10.1007/s10562-020-03323-8
Springer Science and Business Media LLC
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