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Emergence of photoluminescence on bulk MoS by laser thinning and gold particle decoration

Nano Research, ISSN: 1998-0000, Vol: 11, Issue: 9, Page: 4574-4586
2018
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Article Description

We demonstrate a facile and effective approach to significantly improve the photoluminescence of bulk MoS via laser thinning followed by gold particle decoration. Upon laser thinning of exfoliated bulk MoS, photoluminescence emerges from the laser-thinned region. After further treatment with an AuCl solution, gold particles self-assemble on the laser-thinned region and thick edges, further increasing the fluorescence of bulk MoS 28 times and the Raman response 3 times. Such fluorescence enhancement can be attributed to both surface plasmon resonance and p-type doping induced by gold particles. The combination of laser thinning and AuCl treatment enables the functionalization of bulk MoS for optoelectronic applications. It can also provide a viable strategy for mask-free and area-selective p-type doping on single MoS flakes. [Figure not available: see fulltext.].

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