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FTIR study of the interaction of Re 2 (CO) 10 with Na-Y zeolite

Journal of Molecular Catalysis, ISSN: 0304-5102, Vol: 70, Issue: 1, Page: 43-52
1991
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Article Description

The interaction of Re 2 (CO) 10 with zeolite Na-Y was studied by means of FTIR spectroscopy. Three species of supported metal carbonyl were found and assigned to (I) slightly perturbed (physisorbed) Re 2 (CO) 10 molecules, (II) Re 2 (CO) 10 O-bonded to zeolitic Na + ions via a CO ligand and (III) more perturbed Re 2 (CO) 10 molecules encaged inside the faujasite supercages. Upon thermolysis at 630 K the zeolite-supported metal carbonyl was completely decarbonylated. The remaining metal particles were detected spectroscopically by CO adsorption at room temperature.

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