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In situ XPS characterization of the species derived from supported Os carbonyls

Spectrochimica Acta Part A: Molecular Spectroscopy, ISSN: 0584-8539, Vol: 43, Issue: 12, Page: 1497-1501
1987
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The surface reactivity of SiO2-supported Os carbonyl clusters has been followed by in situ treatments in the X-ray photoelectron spectrometer chamber. The mean Os oxidation state in all reported initial systems has been obtained. The effects of exposing to different gases (H 2, O 2, CO, N 2, Ar) and at different temperatures (373-623 K) the samples have been rationalized by comparison with binding energy (b.c.) data for pure Os species [R. Zanoni et al., J. molec. Struct. 131, 363 (1985)] or untreated samples.

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