Supramolecular interaction controlled and calix[4]arene ligand assisted Pd-catalyzed C(sp 3 )−H arylation of aliphatic aldehydes
Chinese Chemical Letters, ISSN: 1001-8417, Vol: 33, Issue: 12, Page: 5116-5119
2022
- 3Citations
- 2Captures
- 1Mentions
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Most Recent News
Researchers from Changzhou University Detail Findings in Supramolecular Research [Supramolecular Interaction Controlled and Calix[4]Arene Ligand Assiste D Pd-catalyzed C(Sp(3))-h Arylation of Aliphatic Aldehydes]
2022 DEC 05 (NewsRx) -- By a News Reporter-Staff News Editor at Nanotech Daily -- New research on Nanotechnology - Supramolecular Research is the subject
Article Description
A calix[4]arene ligand assisted direct β -C−H arylation of tertiary aliphatic aldehydes has been developed via a Pd-catalyzed C(sp 3 )−H functionalization process. This strategy exhibited good functional group compatibility and C−H bond site-selectivity. Mechanism studies have shown that both synergistic effect and cationic- π supramolecular interaction between calixarene cavity and transition-metal catalytic center may play an important role in this catalytic cycle. This complementary method would be used in organic and medical chemistry due to the importance of tertiary aliphatic aldehydes.
Bibliographic Details
http://www.sciencedirect.com/science/article/pii/S1001841722003436; http://dx.doi.org/10.1016/j.cclet.2022.03.125; http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=85128292350&origin=inward; https://linkinghub.elsevier.com/retrieve/pii/S1001841722003436; https://dx.doi.org/10.1016/j.cclet.2022.03.125; http://sciencechina.cn/gw.jsp?action=cited_outline.jsp&type=1&id=7347887&internal_id=7347887&from=elsevier
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