Vibrational energy relaxation of the 7-azaindole dimer in CCl 4 solution studied by picosecond time-resolved transient fluorescence detected IR spectroscopy
Chemical Physics Letters, ISSN: 0009-2614, Vol: 396, Issue: 4, Page: 298-302
2004
- 18Citations
- 21Captures
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Article Description
The picosecond time-resolved IR spectra of the 7-azaindole dimer in a carbon tetrachloride solution was measured by using picosecond time-resolved IR/UV double resonance spectroscopy. This spectroscopy selectively detects the IR transition by transient fluorescence due to an electronic transition from a vibrationally excited level. The time-evolution of the IR spectrum is a single exponential with a 19 ps lifetime, which does not correspond to fast nonstatistical decay due to the intramolecular vibrational redistribution found in a gas-phase cluster. From a comparison with the time-resolved IR spectrum of a jet-cooled dimer, this decay is assigned to vibrational cooling from the dimer to the solvent.
Bibliographic Details
http://www.sciencedirect.com/science/article/pii/S0009261404012394; http://dx.doi.org/10.1016/j.cplett.2004.08.041; http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=7444247369&origin=inward; https://linkinghub.elsevier.com/retrieve/pii/S0009261404012394; https://dx.doi.org/10.1016/j.cplett.2004.08.041
Elsevier BV
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