Magnetic recyclable g-C 3 N 4 /Fe 3 O 4 @MIL-100(Fe) ternary catalyst for photo-Fenton degradation of ciprofloxacin
Journal of Environmental Chemical Engineering, ISSN: 2213-3437, Vol: 10, Issue: 6, Page: 108698
2022
- 39Citations
- 17Captures
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Article Description
The slow Fe(III)/Fe(II) cycle rate seriously limits the photo-Fenton degradation efficiency. In this work, a novel g-C 3 N 4 /Fe 3 O 4 @MIL-100(Fe) ternary heterojunction catalyst was prepared via a facile in-situ route under a mild reaction condition, and was further used as a photo-Fenton catalyst for efficient degradation of ciprofloxacin via the synergistic effect. Compared with g-C 3 N 4 and Fe 3 O 4 @MIL-100(Fe), the composite g-C 3 N 4 /Fe 3 O 4 @MIL-100(Fe) exhibited excellent photo-Fenton catalytic activity for high concentration ciprofloxacin (up to 200 mg L −1 ); approximately 94.7% of CIP was degraded within 120 min light irradiation. It is concluded that g-C 3 N 4 can produce photo-generated electron transfer and further accelerate Fe(III)/Fe(II) cycle, leading to an improvement in the degradation efficiency of ciprofloxacin. In addition, the catalyst presents excellent reusability, whereas the removal efficiency of CIP attained 70.0% after three cycles. This study provided a means to enhance the photo-Fenton activity of Fe-MOFs-based catalysts.
Bibliographic Details
http://www.sciencedirect.com/science/article/pii/S2213343722015718; http://dx.doi.org/10.1016/j.jece.2022.108698; http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=85140584863&origin=inward; https://linkinghub.elsevier.com/retrieve/pii/S2213343722015718; https://dx.doi.org/10.1016/j.jece.2022.108698
Elsevier BV
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