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The effect of high-level waste glass composition on spinel liquidus temperature

Journal of Non-Crystalline Solids, ISSN: 0022-3093, Vol: 384, Page: 32-40
2014
  • 21
    Citations
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  • 20
    Captures
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Metric Options:   Counts1 Year3 Year

Metrics Details

  • Citations
    21
    • Citation Indexes
      21
  • Captures
    20

Article Description

Spinel crystals precipitate in high-level waste glasses containing Fe, Cr, Ni, Mn, Zn, and Ru. The liquidus temperature ( TL ) of spinel as the primary crystallization phase is a function of glass composition, and the spinel solubility ( c 0 ) is a function of both glass composition and temperature ( T ). Previously reported models of TL as a function of composition are based on TL measured directly, which requires laborious experimental procedures. Viewing the curve of c 0 versus T as the liquidus line allows a significant broadening of the composition region for model fitting. This paper estimates TL as a function of composition based on c 0 data obtained with the X-ray diffraction technique.

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