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Tetra-cyanostilbene macrocycle: An effective “turn-on” fluorescence sensor for oxalic acid in aqueous media

Journal of Photochemistry and Photobiology A: Chemistry, ISSN: 1010-6030, Vol: 435, Page: 114307
2023
  • 10
    Citations
  • 0
    Usage
  • 3
    Captures
  • 0
    Mentions
  • 0
    Social Media
Metric Options:   Counts1 Year3 Year

Metrics Details

  • Citations
    10
    • Citation Indexes
      10
  • Captures
    3

Article Description

Although some detection methods for oxalic acid have been reported, the rapid, simple and on-site detection on oxalic acid was rarely presented. In this work, a “turn-on” fluorescence sensor for oxalic acid was realized by the simple and on-site procedure in aqueous media. A tetra-cyanostilbene macrocycle was synthesized by simple “2 + 2” condensation in 72 % yield. It displayed the strong “turn-on” blue fluorescence on selectively detecting oxalic acid among various ions and biomolecules. It possessed the high sensing sensitiveness with the detection limit of 3.82 × 10 −6  M. The sensing mechanism was clarified by pH influence on complexation, fluorescence Jobs’ plot, MS spectra, and 1 H NMR spectra, confirming that non-dissociated oxalic acid was bound in the cavity of the macrocycle based on hydrogen bonds. This sensing ability for oxalic acid was successfully applied in test paper, on-site detection for real samples of taros and rust treatment, suggesting the good application prospect in the rapid, simple and on-site detection for oxalic acid in daily life and industry.

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