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Di- ortho -C H arylation of phenylalanine: A bimetallic interaction between Pd(IV)-Ag(I)

Tetrahedron Letters, ISSN: 0040-4039, Vol: 74, Page: 153158
2021
  • 10
    Citations
  • 0
    Usage
  • 3
    Captures
  • 0
    Mentions
  • 0
    Social Media
Metric Options:   Counts1 Year3 Year

Metrics Details

  • Citations
    10
    • Citation Indexes
      10
  • Captures
    3

Article Description

The direct di -ortho -arylation of substituted phenylalanines has been accomplished via methoxyiminoacyl (MIA)-mediated Pd-catalyzed C H functionalization. A diverse array of phenylalanine substrates is amenable to this protocol, providing di -ortho -arylated phenylalanine derivatives with good to high efficiency. Computational results revealed that a bimetallic interaction between Pd(IV)-Ag(I) was formed through the localized orbital, which obviously favored the reductive elimination step of the arylation process.

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