Two-dimensional line-shape analysis of photon-echo signal
Chemical Physics Letters, ISSN: 0009-2614, Vol: 314, Issue: 5, Page: 488-495
1999
- 52Citations
- 60Captures
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Article Description
We analyze the two-dimensional (2D) line shape obtained by 2D Fourier transforming the time-domain response of a photon-echo signal as a function of the two coherence periods, t 1 and t 3. The line shape obtained for a two-level system with homogeneous and inhomogeneous broadening is shown to be sensitive to the magnitude of both of these line-broadening mechanisms. It is shown that the ellipticity of the 2D line shape can be related to the ratio of homogeneous to inhomogeneous broadening.
Bibliographic Details
http://www.sciencedirect.com/science/article/pii/S0009261499011732; http://dx.doi.org/10.1016/s0009-2614(99)01173-2; http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=0000269360&origin=inward; https://linkinghub.elsevier.com/retrieve/pii/S0009261499011732; http://linkinghub.elsevier.com/retrieve/pii/S0009261499011732; http://api.elsevier.com/content/article/PII:S0009261499011732?httpAccept=text/xml; http://api.elsevier.com/content/article/PII:S0009261499011732?httpAccept=text/plain; http://dx.doi.org/10.1016/s0009-2614%2899%2901173-2; https://dx.doi.org/10.1016/s0009-2614%2899%2901173-2
Elsevier BV
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