A hybrid macrocycle with a pyridine subunit displays aromatic character upon uranyl cation complexation
Journal of the American Chemical Society, ISSN: 1520-5126, Vol: 136, Issue: 11, Page: 4281-4286
2014
- 57Citations
- 53Captures
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Metrics Details
- Citations57
- Citation Indexes57
- 57
- CrossRef46
- Captures53
- Readers53
- 53
Article Description
Reported here is a new hybrid macrocycle, cyclo[1]furan[1]pyridine[4] pyrrole (1), that bears analogy to the previously reported mixed heterocycle system cyclo[2]pyridine[4]pyrrole (2) and cyclo[6]pyrrole 3, an all-pyrrole 22 π-electron aromatic expanded porphyrin. The oxidized, dianionic form of 1, [1 - 4H], has been characterized as its uranyl complex. In contrast to 2 and 3 and in spite of the presence of a 2,6-disubstituted pyridine subunit, the uranyl complex of [1 - 4H] displays solid-state structural and solution-phase spectroscopic features consistent with contributions to the overall electronic structure that involve a conjugated, (4n + 2) π-electron aromatic periphery. © 2014 American Chemical Society.
Bibliographic Details
American Chemical Society (ACS)
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