Electroreduction of chlorine gas at platinum electrodes in several room temperature ionic liquids: Evidence of strong adsorption on the electrode surface revealed by unusual voltammetry in which currents decrease with increasing voltage scan rates
Journal of Physical Chemistry C, ISSN: 1932-7447, Vol: 112, Issue: 49, Page: 19477-19483
2008
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Article Description
Voltammetry is reported for chlorine, Cl, dissolved in various room temperature ionic liquids using platinum microdisk electrodes. A single reductive voltammetric wave is seen and attributed to the two-electron reduction of chlorine to chloride. Studies of the effect of voltage scan rate reveal uniquely unusual behavior in which the magnitude of the currents decrease with increasing scan rates. A model for this is proposed and shown to indicate the presence of strongly adsorbed species in the electrode reaction mechanism, most likely chlorine atoms, Cl·. © 2008 American Chemical Society.
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