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Highly electron-deficient hexaazapentacenes and their dihydro precursors

Organic Letters, ISSN: 1523-7060, Vol: 14, Issue: 16, Page: 4190-4193
2012
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Novel silylethynylated N-heteropentacenes that have three adjacent pyrazine rings at the center of a pentacene backbone are reported. These hexaazapentacenes exhibit a record low energy level of lowest unoccupied molecular orbital (LUMO) for N-heteropentacenes and thus are able to oxidize dihydroanthracene to anthracene. Their synthetic precursors are the corresponding dihydrohexaazapentacenes, which exhibit interesting H-bonding. © 2012 American Chemical Society.

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