Matrix-isolation and computational study of salicylhydroxamic acid and its photochemical degradation
Physical Chemistry Chemical Physics, ISSN: 1463-9076, Vol: 7, Issue: 9, Page: 1960-1965
2005
- 12Citations
- 2Captures
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Metrics Details
- Citations12
- Citation Indexes12
- 12
- CrossRef9
- Captures2
- Readers2
Article Description
The IR absorption spectrum of salicylhydroxamic acid (sha) isolated in an argon matrix at 12-21 K has been recorded. Calculations of all the possible entgegen and zusammen keto conformers of sha have been performed at the B3LYP/6-311++G(d,p) level of theory. The computed energies, optimized structures, and relative abundances show that sha exists in the matrix as the z,z,z,z-conformer [relative to the C-O(-H), C-C(-N), C-N and N-O bonds, respectively] and is stabilized by two intramolecular H-bonds. Photofragmentation of the compound in matrix and methanol-water solution has been obtained by irradiation with visible and ultraviolet light. o-Hydroxyphenylisocyanate is the main photolysis product in an argon matrix, while salicylamide is the primary photolysis product in methanol-water solution. © The Owner Societies 2005.
Bibliographic Details
http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=18844400821&origin=inward; http://dx.doi.org/10.1039/b418033j; http://www.ncbi.nlm.nih.gov/pubmed/19787899; https://xlink.rsc.org/?DOI=b418033j; https://dx.doi.org/10.1039/b418033j; https://pubs.rsc.org/en/content/articlelanding/2005/cp/b418033j
Royal Society of Chemistry (RSC)
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