Charge transfer from cobaltammine complex cations to metal fluoride anions in molecular solids with novel photoelectronic effects (metal: Zirconium, titanium)
Dalton Transactions, ISSN: 1477-9234, Vol: 43, Issue: 37, Page: 14039-14044
2014
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Article Description
[Co(en)](TiF) containing H-bonded assembly of a discrete cobaltammine complex cation and titanium fluoride anion was successfully synthesized under solvothermal conditions. A novel photoelectronic effect was observed in the near-UV region. By extending our understanding of this compound, taking into account our previously reported three cobalt complex-containing zirconium fluorides, the mechanism of photoelectronic effects from these molecular solids was determined by investigating the relative work function for their component species with the help of a Scanning Kelvin probe. The results suggest that the charge transfer from the excited cobaltammine complex cations to the metal fluoride anions as a result of the cooperative behaviors might occur upon illumination, which is responsible for these novel photoelectronic effects. © 2014 the Partner Organisations.
Bibliographic Details
http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=84906710736&origin=inward; http://dx.doi.org/10.1039/c4dt01543f; http://www.ncbi.nlm.nih.gov/pubmed/25157680; https://xlink.rsc.org/?DOI=C4DT01543F; http://xlink.rsc.org/?DOI=C4DT01543F; http://pubs.rsc.org/en/content/articlepdf/2014/DT/C4DT01543F; https://dx.doi.org/10.1039/c4dt01543f; https://pubs.rsc.org/en/content/articlelanding/2014/dt/c4dt01543f
Royal Society of Chemistry (RSC)
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