Temperature identification on two 3D Mn(ii) metal-organic frameworks: Syntheses, adsorption and magnetism
RSC Advances, ISSN: 2046-2069, Vol: 4, Issue: 39, Page: 20605-20611
2014
- 19Citations
- 22Captures
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Article Description
Two new 3-D NaCl-type frameworks of [AmineH][Mn(HCOO) ] (AmineH = N(CH) for 1 and AmineH = NH for 2) have been synthesized at different temperatures. The N(CH) cation was generated in situ by the decomposition of a large number of DMF molecules. The potential porosity of the coordination framework of 1 has been estimated using a computational method based on Connolly's algorithm, indicating that compound 1 presents a kinetic radius greater than 1.61 Å. Because unremovable guest cations are clogged in the channels, 1 presents no significant adsorption for CO gas upon desolvation by long-duration thermal activation. In addition, the magnetic behavior of the two compounds was explored. This journal is © the Partner Organisations 2014.
Bibliographic Details
Royal Society of Chemistry (RSC)
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