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Demonstration of efficient electrochemical biogas reforming in a solid oxide electrolyser with titanate cathode

RSC Advances, ISSN: 2046-2069, Vol: 4, Issue: 72, Page: 38474-38483
2014
  • 12
    Citations
  • 0
    Usage
  • 30
    Captures
  • 0
    Mentions
  • 0
    Social Media
Metric Options:   Counts1 Year3 Year

Metrics Details

  • Citations
    12
    • Citation Indexes
      12
  • Captures
    30

Article Description

Biogas reforming is a renewable and promising way to produce syngas. In this work, we demonstrate a novel strategy to directly and electrochemically convert CH-CO into H-CO. Electrochemical reforming of dry CH-CO (1 : 1) mixture is successfully achieved in a 10 μm-thick titanate cathode with oxygen byproduct generated in anode in an oxide-ion-conducting solid oxide electrolyser under external voltages. In addition, loading iron nanocatalyst in titanate cathode or/and increasing applied voltages has further improved CH-CO conversion. The highest methane conversion of approximately 80% is demonstrated for direct electrochemical reforming in cathode in contrast to the low conversion under open circuit condition in oxide-ion-conducting solid oxide electrolyser cathode. © the Partner Organisations 2014.

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