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Rhodium-catalyzed C-H activation of hydrazines leads to isoquinolones with tunable aggregation-induced emission properties

Chemical Communications, ISSN: 1364-548X, Vol: 51, Issue: 76, Page: 14365-14368
2015
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Article Description

Using an internally oxidizing directing group (DG) strategy, we report a Rh-catalyzed synthesis of isoquinolones via C-H activation/annulation of benzoylhydrazines and alkynes. Tunable double cascade cyclization of benzoylhydrazines with two equivalents of alkynes led to tetracyclic amides. These N-heterocycles demonstrated adjustable AIE properties.

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