Determination of the positions of aluminum atoms introduced into SSZ-35 and the catalytic properties of the generated Brønsted acid sites
Physical Chemistry Chemical Physics, ISSN: 1463-9076, Vol: 19, Issue: 9, Page: 6508-6518
2017
- 2Citations
- 6Captures
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Article Description
The positions of aluminum (Al) atoms in SSZ-35 together with the characteristics of the generated protons were investigated by Al multiple quantum magic-angle spinning (MQ-MAS), Si MAS, and H MAS NMR data analyses accompanied by a variable temperature H MAS NMR analysis. The origin of the acidic -OH groups (Brønsted acid sites) generated by introducing Al atoms into the T sites was investigated and the T sites introduced into the Al atoms were revealed. To further determine the catalytic properties of the acidic protons generated in SSZ-35, the influence of the concentration of the Al atoms on the catalytic activity and selectivity during the transformation of toluene was examined.
Bibliographic Details
http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=85027267284&origin=inward; http://dx.doi.org/10.1039/c6cp08143f; http://www.ncbi.nlm.nih.gov/pubmed/28197567; http://xlink.rsc.org/?DOI=C6CP08143F; http://pubs.rsc.org/en/content/articlepdf/2017/CP/C6CP08143F; https://xlink.rsc.org/?DOI=C6CP08143F; https://dx.doi.org/10.1039/c6cp08143f; https://pubs.rsc.org/en/content/articlelanding/2017/cp/c6cp08143f
Royal Society of Chemistry (RSC)
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