Solution synthesis of conveyor-like MnSe nanostructured architectures with an unusual core/shell magnetic structure
CrystEngComm, ISSN: 1466-8033, Vol: 19, Issue: 24, Page: 3331-3337
2017
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Article Description
We report for the first time one-dimensional (1D) wurtzite (WZ) MnSe nanoconveyors with a single-crystalline configuration fabricated by a solution-processed colloidal method. High-resolution transmission electron microscopy (HRTEM) measurements show that the stem of MnSe nanoconveyors grows along the [1100] direction, while the teeth grow along the [0001] direction. We find that the initial WZ nanobelts with the [1100] growth direction are crucial to the formation of nanoconveyors, whereas the teeth are a result of a self-catalyzed growth process induced by the Mn-terminated (0001) surface. The magnetic measurements suggest that 1D WZ MnSe nanoconveyors consist of an antiferromagnetic core and a ferromagnetic shell below the blocking temperature. Furthermore, the hysteresis measurements indicate that these nanoconveyors have 300 Oe coercive fields, which is attributed to the high surface-to-volume ratio of the nanoconveyors. This facile solution-based strategy can be anticipated to synthesize WZ metal chalcogenide nanomaterials with 1D hierarchical structures, for potential applications from spintronics to photocatalysis.
Bibliographic Details
http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=85021636186&origin=inward; http://dx.doi.org/10.1039/c7ce00491e; https://xlink.rsc.org/?DOI=C7CE00491E; http://xlink.rsc.org/?DOI=C7CE00491E; http://pubs.rsc.org/en/content/articlepdf/2017/CE/C7CE00491E; https://dx.doi.org/10.1039/c7ce00491e; https://pubs.rsc.org/en/content/articlelanding/2017/ce/c7ce00491e
Royal Society of Chemistry (RSC)
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