Red to white polymer light-emitting diode (PLED) based on Eu-Zn-Gd-containing metallopolymer
Journal of Materials Chemistry C, ISSN: 2050-7526, Vol: 5, Issue: 19, Page: 4780-4787
2017
- 27Citations
- 14Captures
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Article Description
Through terpolymerization of the red-light complex monomer [Eu(tta)(4-vp-2,2′bpy)] (2; Htta = 2-thenoyltrifluoroacetone; 4-vp-2,2′-bpy = 2-(pyridin-2-yl)-5-(4-vinylphenyl)pyridine), blue-green-light complex monomer [Zn(L)(4-vinyl-Py)Gd(NO)] (8; Salen-type HL = N,N′-bis(3-methoxy-salicylidene)phenylene-1,2-diamine; 4-vinyl-Py = 4-vinyl-pyridine) with MMA (methyl methacrylate), the obtained Eu-Zn-Gd-containing metallopolymer Poly(2-co-MMA-co-8) (120 : 1[2/8 = 2 : 1 or 1 : 2]) exhibits stoichiometry-dependent color-tuning photoluminescence due to effective Zn-Gd-Salen to Eu energy transfer. Moreover, using them as the corresponding emitting layers, a high color-purity red-light polymer light-emitting diode (PLED) with a luminous efficiency of 0.037 lm W and first-example Ln-containing-metallopolymer-based WPLED with an eternal quantum yield of 0.003% is realized.
Bibliographic Details
http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=85021778544&origin=inward; http://dx.doi.org/10.1039/c7tc01054k; https://xlink.rsc.org/?DOI=C7TC01054K; http://xlink.rsc.org/?DOI=C7TC01054K; http://pubs.rsc.org/en/content/articlepdf/2017/TC/C7TC01054K; https://dx.doi.org/10.1039/c7tc01054k; https://pubs.rsc.org/en/content/articlelanding/2017/tc/c7tc01054k
Royal Society of Chemistry (RSC)
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