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Iridium(i) complexes with bidentate NHC ligands as catalysts for dehydrogenative directed C-H silylation

Chemical Communications, ISSN: 1364-548X, Vol: 59, Issue: 28, Page: 4193-4196
2023
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Article Description

A series of (NHC)(cod)Ir(i) complexes bearing NHC-carboxylate ligands were efficiently synthesized and fully characterized. Their solid-state structures confirmed the bidentate coordination mode of these LX-type NHC ligands. These unprecedented iridium(i) complexes demonstrated efficient catalytic activities in dehydrogenative directed C-H silylation of arenes, and allowed for excellent ortho-selectivity control with aromatic silylating agents.

Bibliographic Details

Manguin, Romane; Galiana-Cameo, María; Kittikool, Tanakorn; Barthes, Cécile; Thongpaen, Jompol; Bancal, Etienne; Mallet-Ladeira, Sonia; Yotphan, Sirilata; Castarlenas, Ricardo; Mauduit, Marc; Sortais, Jean-Baptiste; Baslé, Olivier

Royal Society of Chemistry (RSC)

Materials Science; Chemical Engineering; Chemistry

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