Catalytic amination of lactic acid using Ru-zeolites
Dalton Transactions, ISSN: 1477-9234, Vol: 51, Issue: 28, Page: 10773-10778
2022
- 10Citations
- 9Captures
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Example: if you select the 1-year option for an article published in 2019 and a metric category shows 90%, that means that the article or review is performing better than 90% of the other articles/reviews published in that journal in 2019. If you select the 3-year option for the same article published in 2019 and the metric category shows 90%, that means that the article or review is performing better than 90% of the other articles/reviews published in that journal in 2019, 2018 and 2017.
Citation Benchmarking is provided by Scopus and SciVal and is different from the metrics context provided by PlumX Metrics.
Metrics Details
- Citations10
- Citation Indexes10
- 10
- CrossRef5
- Captures9
- Readers9
Article Description
In this work we investigate the synthesis of alanine from lactic acid, a biobased platform chemical, using ammonia as a nitrogen source and Ru/zeolite catalysts. We report a high alanine selectivity when using Ru/BEA of 80-93%. Reaction side products were identified as ethanol, propionic acid or propanamide and the reaction mechanism was investigated. We further optimised reaction conditions resulting in turn over numbers five times higher than previously reported and could reduce Ru leaching by 30-40%. However, leaching and catalyst stability remains a concern. Furthermore, we critically analyse the benefits of Ru/zeolites versus their stability under the basic, high temperature reaction conditions.
Bibliographic Details
http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=85134720703&origin=inward; http://dx.doi.org/10.1039/d2dt00054g; http://www.ncbi.nlm.nih.gov/pubmed/35510805; https://xlink.rsc.org/?DOI=D2DT00054G; https://dx.doi.org/10.1039/d2dt00054g; https://pubs.rsc.org/en/content/articlelanding/2022/dt/d2dt00054g
Royal Society of Chemistry (RSC)
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