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Synthesis of para-Quinone Methides via Oxidative Ring-Opening of Spiro-cyclopropanyl-cyclohexadienones

Synthesis (Germany), ISSN: 1437-210X, Vol: 54, Issue: 21, Page: 4802-4809
2022
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Article Description

An efficient and simple IBX-promoted oxidative ring-opening of spiro-cyclopropanyl-cyclohexadienones was developed. Disubstituted para-quinone methides were obtained with good to excellent yields and high regioselectivity (33 examples, 45-90% yields). This convenient transformation provides a new method to construct significant para-quinone methides and features high efficiency, broad substrate scope, and good functional group compatibility.

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