On the actinic wavelength dependence of OClO photochemistry in solution
Journal of Chemical Physics, ISSN: 0021-9606, Vol: 118, Issue: 4, Page: 1883-1890
2003
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Article Description
The role of actinic wavelength in OClO photochemistry was explored using femtosecond pump-probe spectroscopy. Specifically, the evolution of optical density was monitored at probe wavelengths from 267 to 900 nm following 355-nm photoexcitation of OClO dissolved in water and acetonitrile. A central result was that the extent of geminate recombination in a given solvent is dependent on the interplay between the rate of excited-state vibrational relaxation versus the energy needed to overcome the energy barrier to dissociation.
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