Lattice models of ionic systems with charge asymmetry
Journal of Chemical Physics, ISSN: 0021-9606, Vol: 118, Issue: 14, Page: 6394-6402
2003
- 19Citations
- 9Captures
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Article Description
A thermodynamic investigation of charge-asymmetric lattice models of electrolytes is presented. By explicitly including the clustering of oppositely charged particles and ion-cluster interactions, phase diagrams for 2:1 and 3:1 lattice electrolytes are obtained, and the critical point for the 4:1 ionic system is located. Thus, the results accord well with the trend obtained in recent Monte Carlo simulations and the continuum DHBjCI theory.
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