Molecular dissociation and vibrational excitation in the surface scattering of (N) and (O) clusters
Journal of Chemical Physics, ISSN: 0021-9606, Vol: 119, Issue: 14, Page: 7451-7460
2003
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Article Description
Molecular N and O vibrational excitation and molecular dissociation induced by cluster-surface impact were investigated by means of molecular dynamics simulations. Cluster-surface scattering was simulated under typical experimental conditions, and vibrational excitation and molecular dissociation were monitored for various cluster sizes and incident velocities. Focus was on the influence of surface-to-cluster heat transfer on the molecular product energy distributions.
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