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Theory of exciton-photon interaction in polymers: Polariton spectra of polydiacetylenes

The Journal of Chemical Physics, ISSN: 0021-9606, Vol: 85, Issue: 1, Page: 611-615
1986
  • 18
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Metrics Details

  • Citations
    18
    • Citation Indexes
      18
  • Captures
    11

Article Description

A first principles method will be presented for the calculation of quasiparticle eigenstates in a polymer crystal strongly interacting with electromagnetic radiation. The matter field will be represented by delocalized excitons whose energy spectrum and wavefunction will be determined with the help of the ab initio Green's function formalism of charge transfer exciton theory. The method has been applied for the computation of bulk polariton bands in highly conducting polydiacetylene crystals. © 1986 American Institute of Physics.

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