Spin uncoupling in A CS studied by high-resolution Zeeman and hyperfine quantum beat spectroscopy
The Journal of Chemical Physics, ISSN: 0021-9606, Vol: 96, Issue: 12, Page: 8761-8769
1992
- 18Citations
- 3Captures
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Article Description
The magnetic properties of the B spin component of the A state in the molecule CS have been investigated with a resolution of ∼ 100 kHz by quantum beat spectroscopy in a supersonic jet. Zeeman-level tuning in CS and CS, providing Landé g factors, and measurements of the CS nuclear hyperfine structure were carried out, particularly to investigate their J dependence. Based on these results, it is proposed that both the magnetic moment and the hyperfine splitting are dominated by spin-uncoupling interactions, described in the rotational Hamiltonian by B( J - S). In addition, the g factors and rotational state lifetimes were used to provide spectroscopic assignments and to elucidate details of the state mixing. © 1992 American Institute of Physics.
Bibliographic Details
http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=0001162813&origin=inward; http://dx.doi.org/10.1063/1.462283; https://pubs.aip.org/jcp/article/96/12/8761/96902/Spin-uncoupling-in-3A2-CS2-studied-by-high; http://aip.scitation.org/doi/10.1063/1.462283; https://aip.scitation.org/action/captchaChallenge?redirectUrl=https%3A%2F%2Faip.scitation.org%2Fdoi%2F10.1063%2F1.462283
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