The insulator to correlated metal phase transition in molybdenum oxides
Applied Physics Letters, ISSN: 0003-6951, Vol: 103, Issue: 5
2013
- 11Citations
- 30Captures
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Article Description
In sub-stoichiometric MoO, electrical and optical responses across the solar spectrum are tunable and manifest a sharp phase transition in thin films at a specific oxygen content. Models of optical response in insulating and conducting regimes have been developed. Oxygen vacancies induce semiconducting response exactly proportional to the observed concentration of gap d-states until the transition. Ionization potential is thus tunable. Metallic thin films are never plasmonic at any stoichiometry and their conductivity, Hall mobility, carrier density, and plasma frequency are consistent, but either loss rate or effective mass mean metallic conduction is correlated rather than classical. © 2013 AIP Publishing LLC.
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