Transient phases during fast crystallization of organic thin films from solution
APL Materials, ISSN: 2166-532X, Vol: 4, Issue: 1
2016
- 20Citations
- 44Captures
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Article Description
We report an in situ microbeam grazing incidence X-ray scattering study of 2,7-dioctyl[1]benzothieno[3,2-b][1]benzothiophene (C-BTBT) organic semiconductor thin film deposition by hollow pen writing. Multiple transient phases are observed during the crystallization for substrate temperatures up to 93 °C. The layered smectic liquid-crystalline phase of C-BTBT initially forms and preceedes inter-layer ordering, followed by a transient crystalline phase for temperature >60 °C, and ultimately the stable phase. Based on these results, we demonstrate a method to produce extremely large grain size and high carrier mobility during high-speed processing. For high writing speed (25 mm/s), mobility up to 3.0 cm/V-s has been observed.
Bibliographic Details
http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=84954122178&origin=inward; http://dx.doi.org/10.1063/1.4939464; https://pubs.aip.org/aip/apm/article-lookup/doi/10.1063/1.4939464; http://dx.doi.org/10.1063/1.4939464.1; https://pubs.aip.org/apm/article/4/1/016103/120881/Transient-phases-during-fast-crystallization-of; http://dx.doi.org/10.1063/1.4939464.3; http://dx.doi.org/10.1063/1.4939464.2
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