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Communication: Approaching exact quantum chemistry by cluster analysis of full configuration interaction quantum Monte Carlo wave functions

Journal of Chemical Physics, ISSN: 0021-9606, Vol: 149, Issue: 15, Page: 151101
2018
  • 65
    Citations
  • 0
    Usage
  • 33
    Captures
  • 0
    Mentions
  • 73
    Social Media
Metric Options:   Counts1 Year3 Year

Metrics Details

  • Citations
    65
  • Captures
    33
  • Social Media
    73
    • Shares, Likes & Comments
      73
      • Facebook
        73

Article Description

We propose to accelerate convergence toward full configuration interaction (FCI) energetics by using the coupled-cluster approach, in which singly and doubly excited clusters, needed to determine the energy, are iterated in the presence of their three- and four-body counterparts extracted from FCI quantum Monte Carlo (FCIQMC) propagations. Preliminary calculations for the water molecule at the equilibrium and stretched geometries show that we can accurately extrapolate the FCI energetics based on the early stages of FCIQMC propagations.

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